Molecular Nanomagnets as Qubits with Embedded Quantum-Error Correction

J Phys Chem Lett. 2020 Oct 15;11(20):8610-8615. doi: 10.1021/acs.jpclett.0c02213. Epub 2020 Sep 29.

Abstract

We show that molecular nanomagnets have a potential advantage in the crucial rush toward quantum computers. Indeed, the sizable number of accessible low-energy states of these systems can be exploited to define qubits with embedded quantum error correction. We derive the scheme to achieve this crucial objective and the corresponding sequence of microwave/radiofrequency pulses needed for the error correction procedure. The effectiveness of our approach is shown already with a minimal S = 3/2 unit corresponding to an existing molecule, and the scaling to larger spin systems is quantitatively analyzed.