Iterative learning control (ILC) can synthesize the feedforward control signal for the trajectory tracking control of a repetitive task, even when the system has strong nonlinear dynamics. This makes ILC be one of the most popular methods for trajectory tracking control. Restriction on a repetitive task, however, limits its application to multiple trajectories. This article proposes a neural-network-based ILC (NN-ILC) to deal with nonrepetitive tasks very effectively. A position-based ILC is designed to compensate the tracking error, based on which the multiple outputs of the ILC (ILC outputs) for multiple tasks are expressed as a function of the reference position, velocity, and acceleration. The proposed NN-ILC divides the ILC outputs of multiple tasks into two parts: the linear and nonlinear portions. The first part is expressed by a linear function, which is the linear portion of the function of the ILC outputs. The second part is expressed by a nonlinear function, which is estimated by complementary neural networks including a general neural network and a switching neural network. Finally, the two parts are combined and the ILC outputs of multiple tasks are expressed as a neural-network-based function. Two advantages of the proposed NN-ILC are emphasized. First, the ILC outputs of multiple tasks are compressed into a function by the proposed method, and thus, the memories can be saved. Second, in terms of generalizability, the neural-network-based function of the ILC outputs can easily predict position compensation for multiple tasks without extra iterative learning processes. Experimental results on a robot arm show that the proposed NN-ILC method can easily realize the ILC of multiple tasks. It can save memory comparing with the method of storing the data of multiple tasks and can predict the ILC output of any task, which can accelerate the iterative learning process.