Exchange-coupled nanocomposites are considered as the most promising materials for production of high-energy performance permanent magnets, which can exceed neodymium ones in terms of energy product. In this work, micromagnetic simulations of L10-FeNi/SmCo5 composites based on the initially anisotropic structure of nanorods array were performed. Texturing effect on magnetic properties was investigated. It was revealed that even 30% of anisotropy axes misalignment of grains in L10-FeNi phase would lead to only ≈10% drop of coercivity. To maximize magnetic properties of the composites, parameters of microstructure were optimized for 120 × 120 array of interacting nanorods and were found to be 40 nm nanorod diameter and 12-20 nm interrod distance. The estimated diameter of nanorods and the packing density of the array provide energy product values of 149 kJ m-3. Influence of interrod distance on energy product values was explored. Approaches for production of exchange-coupled composites based on anisotropic nanostructures were proposed.