Superconductivity in Single-Quintuple-Layer Bi2Te3 Grown on Epitaxial FeTe

Nano Lett. 2020 May 13;20(5):3160-3168. doi: 10.1021/acs.nanolett.9b05167. Epub 2020 Mar 31.

Abstract

How an interfacial superconductivity emerges during the nucleation and epitaxy is of great importance not only for unveiling the physical insights but also for finding a feasible way to tune the superconductivity via interfacial engineering. In this work, we report the nanoscale creation of a robust and relatively homogeneous interfacial superconductivity (TC ≈ 13 K) on the epitaxial FeTe surface, by van der Waals epitaxy of single-quintuple-layer topological insulator Bi2Te3. Our study suggests that the superconductivity in the Bi2Te3/FeTe heterostructure is generated at the interface and that the superconductivity at the interface does not enhance or weaken with the increase of the Bi2Te3 thickness beyond 1 quintuple layer (QL). The observation of the topological surface states crossing Fermi energy in the Bi2Te3/FeTe heterostructure with the average Bi2Te3 thickness of about 20 QL provides further evidence that this heterostructure may potentially host Majorana zero modes.

Keywords: FeTe/Bi2Te3; charge transfer; interfacial superconductivity; scanning tunneling microscopy; step-flow epitaxy.