One-dimensional nanomaterials, including both nanowires (NWs) and nanotubes (NTs), have been extensively investigated in the decades because of their unique physicochemical properties. Particularly, aligning NWs/NTs into a network or complex micropatterns has been a key issue for its unique integrated functionalities, which enjoy benefits in versatile applications. So far, solution processes remain the most effective strategy to align NWs/NTs, which also bear advantages of mild operation condition and large-scale production. In this perspective, particular attention is drawn to the currently widely used solution coating approaches for aligning NWs/NTs, including the Langmuir-Blodgett film technique, solution shearing approaches, and methods of tri-phase contact line manipulation. We also proposed several perspectives in this field.