A Single-Crystalline Silver Plasmonic Circuit for Visible Quantum Emitters

Nano Lett. 2019 May 8;19(5):3238-3243. doi: 10.1021/acs.nanolett.9b00773. Epub 2019 Apr 26.

Abstract

Plasmonic waveguides are key elements in nanophotonic devices, serving as optical interconnects between nanoscale light sources and detectors. Multimode operation in plasmonic two-wire transmission lines promises important degrees of freedom for near-field manipulation and information encoding. However, highly confined plasmon propagation along gold nanostructures is typically limited to the near-infrared region due to ohmic losses, excluding all visible quantum emitters from plasmonic circuitry. We report on the top-down fabrication of complex plasmonic nanostructures in single-crystalline silver plates. We demonstrate the controlled remote excitation of a small ensemble of fluorophores by a set of waveguide modes and the emission of the visible luminescence into the waveguide with high efficiency. This approach opens up the study of a nanoscale light-matter interaction between complex plasmonic waveguides and a large variety of quantum emitters available in the visible spectral range.

Keywords: Two-wire gap-plasmon waveguide; focused ion beam milling; molecular fluorescence; nanocircuit; silver flake; silver nanowire.

Publication types

  • Research Support, Non-U.S. Gov't