Stretchable Electroluminescent Display Enabled by Graphene-Based Hybrid Electrode

ACS Appl Mater Interfaces. 2019 Apr 17;11(15):14222-14228. doi: 10.1021/acsami.8b22135. Epub 2019 Apr 5.

Abstract

Stretchable alternating-current electroluminescent (ACEL) devices are required due to their potential in wearable, biomedical, e-skin, robotic, lighting, and display applications; however, one of the main hurdles is to achieve uniform electroluminescence with an optimal combination of transparency, conductivity, and stretchability in electrodes. We therefore propose a fabrication scheme involving strategically combining two-dimensional graphene layers with a silver nanowire (Ag NW)-embedded PEDOT:PSS film. The developed hybrid electrode overcomes the limitations of commonly known metallic NWs and ionic conductor-based electrodes for ACEL applications. Furthermore, the potential of the hybrid electrode is realized in demonstrating large-area stretchable ACEL devices composed of an 8 × 8 passive array. The prototype ACEL passive array demonstrates efficient and uniform electroluminescence under high levels of mechanical deformation such as bending, rolling, twisting, and stretching.

Keywords: PEDOT:PSS; ZnS; alternating-current electroluminescence device; graphene; silver nanowires; stretchable display; stretchable electrode.