Terraced and Smooth Gradient Polymer Brushes via a Polymer Single-Crystal Assisted Grafting-To Method

Angew Chem Int Ed Engl. 2018 Nov 26;57(48):15758-15761. doi: 10.1002/anie.201809915. Epub 2018 Oct 31.

Abstract

Gradient polymer brushes provide a spatial gradient change in molecular characteristics of the brush, and such a change can be utilized to study structure-property relationships in a combinatorial fashion. In this study, a bottom-up method was used to synthesize gradient polymer brushes with a predesigned and precisely controlled grafting density gradient and brush pattern. A polymer single-crystal assisted grafting-to (PSCAGT) method was employed where end-functionalized polymers were grown into two-dimensional polymer single crystals. The latter were chemically coupled to a solid substrate to form well-defined polymer brushes. To tune the grafting density, end-dissimilar polymers were used to co-crystallize into one single crystal. Programmed single-crystal growth was introduced to synthesize brushes with two different gradient architectures, that is, terraced and smooth gradient with pyramid patterns. This work demonstrates that the PSCAGT method offers a unique means to tune polymer brush nanostructure.

Keywords: gradient brushes; nanopatterning; nanostructures; polymer brushes; polymer crystallization.