Spin-polarized resonant surface state in (1 1 1) Sm1-x Gd x Al2, a zero-magnetization ferromagnet

J Phys Condens Matter. 2018 Oct 31;30(43):435501. doi: 10.1088/1361-648X/aae341. Epub 2018 Sep 21.

Abstract

The electronic structure of (1 1 1) Sm1-x Gd x Al2, a zero-magnetization ferromagnet, is investigated by angle- and spin- resolved photoemission spectroscopy. An intense electron pocket strongly localized around [Formula: see text] and close to the Fermi level is observed and analyzed in detail. Its various characteristics, combined with electronic structure calculations, reveal a resonant surface state of 5d character and Λ1 symmetry, likely built on bulk states developing around L points. It exhibits moreover a low temperature positive spin polarization at the Fermi level, of strong interest for spin-dependent transport properties in Sm1-x Gd x Al2-based spintronic devices.