Non-Markovian decoherence dynamics in nonequilibrium environments

J Chem Phys. 2018 Sep 7;149(9):094107. doi: 10.1063/1.5039891.

Abstract

We theoretically investigate the non-Markovian dynamical decoherence of a quantum system coupled to nonequilibrium environments with nonstationary statistical properties. We show the time evolution of the decoherence factor in real-imaginary space to study the environment-induced energy renormalization and backaction of coherence which are associated with the unitary and nonunitary parts of the quantum master equation, respectively. It is also shown that the nonequilibrium decoherence dynamics displays a transition between Markovian and non-Markovian and the transition boundary depends on the environmental parameters. The results are helpful for further understanding non-Markovian dynamics and coherence backaction on an open quantum system from environments.