Piezotronic Effect Enhanced Flexible Humidity Sensing of Monolayer MoS2

ACS Appl Mater Interfaces. 2018 Mar 7;10(9):8110-8116. doi: 10.1021/acsami.7b17529. Epub 2018 Feb 26.

Abstract

We report the piezotronic effect on the performance of humidity detection based on a back-to-back Schottky contacted monolayer MoS2 device. By introducing an upswept mechanical strain, the in-plane electrical polarization can be induced at the MoS2/metal junction region. The polarization charges can modify the Schottky barrier height at the interface of MoS2/metal junction, subsequently improving the sensitivity of the humidity sensing. An energy band diagram is proposed to explain the experiment phenomenon of the humidity sensor. This work provides a simple way to enhance the sensitivity of ultrathin two-dimensional-materials-based sensors by the piezotronic effect, which has great potential applications in electronic skin, human-computer interfacing, gas sensing, and environment monitoring.

Keywords: Schottky barrier height; humidity sensing; monolayer MoS2; piezotronic effect; polarization charges.