Bosonic Confinement and Coherence in Disordered Nanodiamond Arrays

ACS Nano. 2017 Nov 28;11(11):11746-11754. doi: 10.1021/acsnano.7b07148. Epub 2017 Nov 13.

Abstract

In the presence of disorder, superconductivity exhibits short-range characteristics linked to localized Cooper pairs which are responsible for anomalous phase transitions and the emergence of quantum states such as the bosonic insulating state. Complementary to well-studied homogeneously disordered superconductors, superconductor-normal hybrid arrays provide tunable realizations of the degree of granular disorder for studying anomalous quantum phase transitions. Here, we investigate the superconductor-bosonic dirty metal transition in disordered nanodiamond arrays as a function of the dispersion of intergrain spacing, which ranges from angstroms to micrometers. By monitoring the evolved superconducting gaps and diminished coherence peaks in the single-quasiparticle density of states, we link the destruction of the superconducting state and the emergence of bosonic dirty metallic state to breaking of the global phase coherence and persistence of the localized Cooper pairs. The observed resistive bosonic phase transitions are well modeled using a series-parallel circuit in the framework of bosonic confinement and coherence.

Keywords: amorphous carbon; confinement and coherence; disordered hybrid arrays; nanodiamond; superconducting order parameter.

Publication types

  • Research Support, Non-U.S. Gov't