Historical and future emission of hazardous air pollutants (HAPs) from gas-fired combustion in Beijing, China

Environ Sci Pollut Res Int. 2017 Jul;24(20):16946-16957. doi: 10.1007/s11356-017-9260-6. Epub 2017 Jun 3.

Abstract

The consumption of natural gas in Beijing has increased in the past decade due to energy structure adjustments and air pollution abatement. In this study, an integrated emission inventory of hazardous air pollutants (HAPs) emitted from gas-fired combustion in Beijing was developed for the period from 2000 to 2014 using a technology-based approach. Future emission trends were projected through 2030 based on current energy-related and emission control policies. We found that emissions of primary HAPs exhibited an increasing trend with the rapid increase in natural gas consumption. Our estimates indicated that the total emissions of NO X , particulate matter (PM)10, PM2.5, CO, VOCs, SO2, black carbon, Pb, Cd, Hg, As, Cr, Cu, Ni, Zn, polychlorinated dibenzo-p-dioxins and dibenzofurans, and benzo[a]pyrene from gas-fired combustion in Beijing were approximately 22,422 t, 1042 t, 781 t, 19,097 t, 653 t, 82 t, 19 t, 0.6 kg, 0.1 kg, 43 kg, 52 kg, 0.3 kg, 0.03 kg, 4.3 kg, 0.6 kg, 216 μg, and 242 g, respectively, in 2014. To mitigate the associated air pollution and health risks caused by gas-fired combustion, stricter emission standards must be established. Additionally, combustion optimization and flue gas purification system could be used for lowering NO X emissions from gas-fired combustion, and gas-fired facilities should be continuously monitored based on emission limits. Graphical abstract Spatial distribution and typical live photos of gas-fired boiler in Beijing.

Keywords: Emission inventory; Gas-fired combustion; Hazardous air pollutants (HAPs); Spatial variation; Temporal trends.

MeSH terms

  • Air Pollutants*
  • Air Pollution
  • Beijing
  • China
  • Environmental Monitoring*
  • Particulate Matter

Substances

  • Air Pollutants
  • Particulate Matter