Allosteric Communication Disrupted by a Small Molecule Binding to the Imidazole Glycerol Phosphate Synthase Protein-Protein Interface

Biochemistry. 2016 Nov 29;55(47):6484-6494. doi: 10.1021/acs.biochem.6b00859. Epub 2016 Nov 11.

Abstract

Allosteric enzymes regulate a wide range of catalytic transformations, including biosynthetic mechanisms of important human pathogens, upon binding of substrate molecules to an orthosteric (or active) site and effector ligands at distant (allosteric) sites. We find that enzymatic activity can be impaired by small molecules that bind along the allosteric pathway connecting the orthosteric and allosteric sites, without competing with endogenous ligands. Noncompetitive allosteric inhibitors disrupted allostery in the imidazole glycerol phosphate synthase (IGPS) enzyme from Thermotoga maritima as evidenced by nuclear magnetic resonance, microsecond time-scale molecular dynamics simulations, isothermal titration calorimetry, and kinetic assays. The findings are particularly relevant for the development of allosteric antibiotics, herbicides, and antifungal compounds because IGPS is absent in mammals but provides an entry point to fundamental biosynthetic pathways in plants, fungi, and bacteria.

MeSH terms

  • Allosteric Regulation*
  • Allosteric Site
  • Aminohydrolases / chemistry
  • Aminohydrolases / metabolism*
  • Bacterial Proteins / chemistry
  • Bacterial Proteins / metabolism*
  • Binding Sites
  • Biocatalysis
  • Calorimetry / methods
  • Catalytic Domain
  • Crystallography, X-Ray
  • Imidazoles / chemistry
  • Imidazoles / metabolism
  • Ligands
  • Magnetic Resonance Spectroscopy
  • Molecular Dynamics Simulation
  • Protein Binding
  • Protein Domains
  • Protein Subunits / chemistry
  • Protein Subunits / metabolism
  • Ribonucleotides / chemistry
  • Ribonucleotides / metabolism
  • Small Molecule Libraries / chemistry
  • Small Molecule Libraries / metabolism*
  • Thermotoga maritima / enzymology

Substances

  • Bacterial Proteins
  • Imidazoles
  • Ligands
  • Protein Subunits
  • Ribonucleotides
  • Small Molecule Libraries
  • N(1)-((5'-phosphoribulosyl)formimino)-5-aminoimidazo-4-carboxamide ribonucleotide
  • imidazole glycerol phosphate synthase
  • Aminohydrolases