Proximity-Induced Spin Polarization of Graphene in Contact with Half-Metallic Manganite

ACS Nano. 2016 Aug 23;10(8):7532-41. doi: 10.1021/acsnano.6b02424. Epub 2016 Jul 20.

Abstract

The role of proximity contact with magnetic oxides is of particular interest from the expectations of the induced spin polarization and weak interactions at the graphene/magnetic oxide interfaces, which would allow us to achieve efficient spin-polarized injection in graphene-based spintronic devices. A combined approach of topmost-surface-sensitive spectroscopy utilizing spin-polarized metastable He atoms and ab initio calculations provides us direct evidence for the magnetic proximity effect in the junctions of single-layer graphene and half-metallic manganite La0.7Sr0.3MnO3 (LSMO). It is successfully demonstrated that in the graphene/LSMO junctions a sizable spin polarization is induced at the Fermi level of graphene in parallel to the spin polarization direction of LSMO without giving rise to a significant modification in the π band structure.

Keywords: graphene; half-metals; interface; magnetic oxides; proximity effect; spin polarization; spintronics.

Publication types

  • Research Support, Non-U.S. Gov't