NMR Evidence for Inhomogeneous Nematic Fluctuations in BaFe_{2}(As_{1-x}P_{x})_{2}

Phys Rev Lett. 2016 Mar 11;116(10):107202. doi: 10.1103/PhysRevLett.116.107202. Epub 2016 Mar 10.

Abstract

We present evidence for nuclear spin-lattice relaxation driven by glassy nematic fluctuations in isovalent P-doped BaFe_{2}As_{2} single crystals. Both the ^{75}As and ^{31}P sites exhibit a stretched-exponential relaxation similar to the electron-doped systems. By comparing the hyperfine fields and the relaxation rates at these sites we find that the As relaxation cannot be explained solely in terms of magnetic spin fluctuations. We demonstrate that nematic fluctuations couple to the As nuclear quadrupolar moment and can explain the excess relaxation. These results suggest that glassy nematic dynamics are a common phenomenon in the iron-based superconductors.