Quantitative and Direct Near-Field Analysis of Plasmonic-Induced Transparency and the Observation of a Plasmonic Breathing Mode

ACS Nano. 2016 Feb 23;10(2):2214-24. doi: 10.1021/acsnano.5b06768. Epub 2016 Feb 1.

Abstract

We investigated experimentally and numerically in the optical near-field a plasmonic model system similar to a dolmen-type structure for phenomena such as plasmon-induced transparency. Through engineering of coupling strength, structure orientation, and incident angle and phase of the excitation source it was possible to control near-field excitation of the dark modes. We showed that quantitative analysis of near-field amplitude and excitation strength provided essential information that allowed identifying the interaction between the bright and the dark mode and how it causes the formation of plasmon-induced transparency features and a Fano resonance. In addition, we introduced a mechanism to excite field distributions in plasmonic structures that cannot be accessed directly using far-field illumination and demonstrated the excitation of a dark mode akin to a symmetry-forbidden plasmonic breathing mode using a linearly polarized far-field source.

Keywords: EIT; Fano resonance; PIT; breathing mode; dark modes; plasmonics; scanning near-field optical microscopy.

Publication types

  • Research Support, Non-U.S. Gov't