Fully Printed Halide Perovskite Light-Emitting Diodes with Silver Nanowire Electrodes

Sri Ganesh R Bade; Junqiang Li; Xin Shan; Yichuan Ling; Yu Tian; Tristan Dilbeck; Tiglet Besara; Thomas Geske; Hanwei Gao; Biwu Ma; Kenneth Hanson; Theo Siegrist; Chengying Xu; Zhibin Yu

doi:10.1021/acsnano.5b07506

Fully Printed Halide Perovskite Light-Emitting Diodes with Silver Nanowire Electrodes

ACS Nano. 2016 Feb 23;10(2):1795-801. doi: 10.1021/acsnano.5b07506. Epub 2015 Dec 31.

Authors

Sri Ganesh R Bade^{1

2}, Junqiang Li^{1

2}, Xin Shan^{1

2}, Yichuan Ling^{1

2}, Yu Tian^{1

2}, Tristan Dilbeck^{1

2}, Tiglet Besara^{1

2}, Thomas Geske^{1

2}, Hanwei Gao^{1

2}, Biwu Ma^{1

2}, Kenneth Hanson^{1

2}, Theo Siegrist^{1

2}, Chengying Xu^{1

2}, Zhibin Yu^{1

2}

Affiliations

¹ Department of Industrial and Manufacturing Engineering, High Performance Materials Institute, §Department of Chemical and Biomedical Engineering, #National High Magnetic Field Laboratory, and ⊗Department of Mechanical Engineering, Florida State University , Tallahassee Florida 32310, United States.
² Department of Physics, ∥Department of Chemistry and Biochemistry, and ⊥Materials Science and Engineering, Florida State University , Tallahassee Florida 32306, United States.

PMID: 26713348
DOI: 10.1021/acsnano.5b07506

Abstract

Printed organometal halide perovskite light-emitting diodes (LEDs) are reported that have indium tin oxide (ITO) or carbon nanotubes (CNTs) as the transparent anode, a printed composite film consisting of methylammonium lead tribromide (Br-Pero) and poly(ethylene oxide) (PEO) as the emissive layer, and printed silver nanowires as the cathode. The fabrication can be carried out in ambient air without humidity control. The devices on ITO/glass have a low turn-on voltage of 2.6 V, a maximum luminance intensity of 21014 cd m(-2), and a maximum external quantum efficiency (EQE) of 1.1%, surpassing previous reported perovskite LEDs. The devices on CNTs/polymer were able to be strained to 5 mm radius of curvature without affecting device properties.

Keywords: composites; flexible electronics; halide perovskites; light-emitting diodes; moisture; printed electronics.

Publication types

Research Support, U.S. Gov't, Non-P.H.S.