Solvothermal Synthesis of Lateral Heterojunction Sb2Te3/Bi2Te3 Nanoplates

Nano Lett. 2015 Sep 9;15(9):5905-11. doi: 10.1021/acs.nanolett.5b01987. Epub 2015 Aug 27.

Abstract

A lateral heterojunction of topological insulator Sb2Te3/Bi2Te3 was successfully synthesized using a two-step solvothermal method. The two crystalline components were separated well by a sharp lattice-matched interface when the optimized procedure was used. Inspecting the heterojunction using high-resolution transmission electron microscopy showed that epitaxial growth occurred along the horizontal plane. The semiconducting temperature-resistance curve and crossjunction rectification were observed, which reveal a staggered-gap lateral heterojunction with a small junction voltage. Quantum correction from the weak antilocalization reveals the well-maintained transport of the topological surface state. This is appealing for a platform for spin filters and one-dimensional topological interface states.

Keywords: antimony telluride; bismuth telluride; heterojunction; solvothermal synthesis; topological insulator; transport.

Publication types

  • Research Support, Non-U.S. Gov't