Multiscale Theoretical Modeling of Plasmonic Sensing of Hydrogen Uptake in Palladium Nanodisks

J Phys Chem Lett. 2012 Sep 20;3(18):2556-61. doi: 10.1021/jz3007723. Epub 2012 Aug 30.

Abstract

We study theoretically the optical properties of palladium nanodisks during hydrogen uptake. A combination of an ab initio quantum mechanical description of the Pd-H dielectric properties and a full electrodynamical study of light scattering in the H-modified Pd nanodisks allows us to trace the shift of the localized surface plasmon as a function of the H concentration in the Pd-H disk. We follow the evolution of the plasmon peak energy for different admixtures of the Pd-H α and β phases and interpret quantitatively the experimental sensitivity of the plasmon energy shift to the structural inhomogeneity upon H absorption. Our multiscale theoretical framework provides a solid background for plasmonic sensing of structural domains, as well as for identifying H saturation conditions in metal hydride systems.

Keywords: ab initio calculations; hydrogen sensing; hydrogen storage; palladium hydride; plasmonic sensing; surface plasmon sensing.