Hybridization in Three Dimensions: A Novel Route toward Plasmonic Metamolecules

Nano Lett. 2015 Aug 12;15(8):5200-7. doi: 10.1021/acs.nanolett.5b01437. Epub 2015 Jul 30.

Abstract

Plasmonic metamolecules have received much interest in the last years because they can produce a wide spectrum of different hybrid optical resonances. Most of the configurations presented so far, however, considered planar resonators lying on a dielectric substrate. This typically yields high damping and radiative losses, which severely limit the performance of the system. Here we show that these limits can be overcome by considering a 3D arrangement made from slanted nanorod dimers extruding from a silver baseplate. This configuration mimics an out-of-plane split ring resonator capable of a strong near-field interaction at the terminations and a strong diffractive coupling with nearby nanostructures. Compared to the corresponding planar counterparts, higher values of electric and magnetic fields are found (about a factor 10 and a factor 3, respectively). High-quality-factor resonances (Q ≈ 390) are produced in the mid-IR as a result of the efficient excitation of collective modes in dimer arrays.

Keywords: 3D metamolecule; 3D split ring; Fano lattice resonance; electromagnetic field enhancement; hollow nanoantenna; plasmon hybridization.

Publication types

  • Research Support, Non-U.S. Gov't