Chemical Sensing of 2D Graphene/MoS2 Heterostructure device

ACS Appl Mater Interfaces. 2015 Aug 5;7(30):16775-80. doi: 10.1021/acsami.5b04541. Epub 2015 Jul 22.

Abstract

We report the production of a two-dimensional (2D) heterostructured gas sensor. The gas-sensing characteristics of exfoliated molybdenum disulfide (MoS2) connected to interdigitated metal electrodes were investigated. The MoS2 flake-based sensor detected a NO2 concentration as low as 1.2 ppm and exhibited excellent gas-sensing stability. Instead of metal electrodes, patterned graphene was used for charge collection in the MoS2-based sensing devices. An equation based on variable resistance terms was used to describe the sensing mechanism of the graphene/MoS2 device. Furthermore, the gas response characteristics of the heterostructured device on a flexible substrate were retained without serious performance degradation, even under mechanical deformation. This novel sensing structure based on a 2D heterostructure promises to provide a simple route to an essential sensing platform for wearable electronics.

Keywords: MoS2; flexible device; gas sensor; graphene; heterostructure.

Publication types

  • Research Support, Non-U.S. Gov't