Surface coal mine land reclamation using a dry flue gas desulfurization product: Short-term and long-term water responses

Chemosphere. 2015 Sep:134:459-65. doi: 10.1016/j.chemosphere.2015.05.014. Epub 2015 May 23.

Abstract

Abandoned coal-mined lands are a worldwide concern due to their potential negative environmental impacts, including erosion and development of acid mine drainage. A field study investigated the use of a dry flue gas desulfurization product for reclamation of abandoned coal mined land in USA. Treatments included flue gas desulfurization product at a rate of 280 Mg ha(-1) (FGD), FGD at the same rate plus 112 Mg ha(-1) yard waste compost (FGD/C), and conventional reclamation that included 20 cm of re-soil material plus 157 Mg ha(-1) of agricultural limestone (SOIL). A grass-legume sward was planted after treatment applications. Chemical properties of surface runoff and tile water (collected from a depth of 1.2m below the ground surface) were measured over both short-term (1-4 yr) and long-term (14-20 yr) periods following reclamation. The pH of surface runoff water was increased from approximately 3, and then sustained at 7 or higher by all treatments for up to 20 yr, and the pH of tile flow water was also increased and sustained above 5 for 20 yr. Compared with SOIL, concentrations of Ca, S and B in surface runoff and tile flow water were generally increased by the treatments with FGD product in both short- and long-term measurements and concentrations of the trace elements were generally not statistically increased in surface runoff and tile flow water over the 20-yr period. However, concentrations of As, Ba, Cr and Hg were occasionally elevated. These results suggest the use of FGD product for remediating acidic surface coal mined sites can provide effective, long-term reclamation.

Keywords: Acid mine drainage; Flue gas desulfurization (FGD) product; Surface coal mine reclamation; Trace element; Water quality.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Agriculture
  • Arsenic / analysis
  • Barium / analysis
  • Boron / analysis
  • Calcium / analysis
  • Chromium / analysis
  • Coal / analysis*
  • Conservation of Natural Resources
  • Environmental Monitoring / methods
  • Environmental Restoration and Remediation*
  • Gases
  • Hydrogen-Ion Concentration
  • Mercury / analysis
  • Mining*
  • Soil
  • Soil Pollutants / analysis
  • Sulfur / analysis*
  • Trace Elements / analysis*
  • Water
  • Water Pollutants, Chemical / analysis

Substances

  • Coal
  • Gases
  • Soil
  • Soil Pollutants
  • Trace Elements
  • Water Pollutants, Chemical
  • Water
  • Chromium
  • Barium
  • Sulfur
  • Mercury
  • Arsenic
  • Boron
  • Calcium