Picosecond optical parametric generator and amplifier for large temperature-jump

Opt Express. 2014 Dec 1;22(24):30047-52. doi: 10.1364/OE.22.030047.

Abstract

An optical parametric generator and amplifier producing 15 ps pulses at wavelengths tunable around 2 μm, with energies up to 15 mJ/pulse, has been realized and characterized. The output wavelength is chosen to match a vibrational combination band of water. By measuring the induced birefringence changes we prove that a single pulse is able to completely melt samples of ice in the 10⁻⁶ cm³ volume range, both at room pressure (263 K) and at high pressure (298 K, 1 GPa) in a sapphire anvil cell. This source opens the possibility of studying melting and freezing processes by spectroscopic probes in water or water solutions in a wide range of conditions as found in natural environments.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amplifiers, Electronic*
  • Birefringence
  • Freezing
  • Ice
  • Optical Phenomena*
  • Signal Processing, Computer-Assisted
  • Temperature*
  • Time Factors

Substances

  • Ice