Carbodiimide/NHS derivatization of COOH-terminated SAMs: activation or byproduct formation?

Langmuir. 2014 Apr 29;30(16):4545-50. doi: 10.1021/la5004269. Epub 2014 Apr 16.

Abstract

COOH-terminated self-assembled monolayers (SAMs) are widely used in biosensor technology to bind different amine-containing biomolecules. A covalent amide bond, however, can be achieved only if the carboxylic acids are activated. This activation process usually consists of forming an N-hydroxysuccinimidyl ester (NHS-ester) by consecutively reacting carboxylic acids with a carbodiimide and NHS. Though many papers report using this method,1-8 the experimental conditions vary greatly between them and chemical characterization at this stage is often omitted. Evidence of an efficient activation is therefore rarely shown. Furthermore, recent publications9-11 have highlighted the complexity of this process, with the possible formation of different byproducts. In this paper, we have conducted a study on NHS activation under different conditions with chemical characterization by polarization-modulation infrared reflection-absorption spectroscopy (PM-IRRAS) and time-of-flight secondary ion mass spectroscopy (ToF-SIMS). Our results indicate that the nature of the solvent and carbodiimide and the reactant concentrations play crucial roles in activation kinetics and efficiency.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Biosensing Techniques
  • Carbodiimides / chemistry*
  • Carboxylic Acids / chemistry*
  • Solvents / chemistry
  • Spectrometry, Mass, Secondary Ion
  • Surface Properties

Substances

  • Carbodiimides
  • Carboxylic Acids
  • Solvents