High-field magnetization and magnetoelasticity of single crystalline HoFe5Al7

J Phys Condens Matter. 2014 Apr 2;26(13):136001. doi: 10.1088/0953-8984/26/13/136001. Epub 2014 Mar 13.

Abstract

Magnetization and ultrasound measurements have been performed in pulsed magnetic fields up to 60 T on a ferrimagnetic HoFe5Al7 single crystal (Curie temperature TC = 216 K, compensation point Tcomp = 65 K) with a tetragonal crystal structure of the ThMn12-type. The compound exhibits a high magnetic anisotropy of the easy-plane type. A large anisotropy is also observed within the basal plane having an easy-magnetization direction along the [110] axis with the spontaneous magnetic moment Ms = 2 µB/f.u. at T = 2 K. Along the easy axis, two first-order field-induced magnetic transitions are observed. At both transitions sharp anomalies in the acoustic properties are found. The critical fields of the transitions depend on temperature in a different manner. Within molecular-field theory and using the high-field magnetization data the Ho-Fe inter-sublattice exchange parameter has been determined to be nHoFe ≈ 4 T/µB. The magnetoelasticity has also been probed by magnetization measurements under hydrostatic pressure. TC decreases with a rate dTC/dp = -10 K/GPa, whereas Tcomp increases with dTcomp/dp = 3.5 K/GPa.

Publication types

  • Research Support, Non-U.S. Gov't