Using thermal boundary conditions to engineer the quantum state of a bulk magnet

Proc Natl Acad Sci U S A. 2014 Mar 11;111(10):3689-94. doi: 10.1073/pnas.1316070111. Epub 2014 Feb 24.

Abstract

The degree of contact between a system and the external environment can alter dramatically its proclivity to quantum mechanical modes of relaxation. We show that controlling the thermal coupling of cubic-centimeter-sized crystals of the Ising magnet LiHo(x)Y(1-x)F4 to a heat bath can be used to tune the system between a glassy state dominated by thermal excitations over energy barriers and a state with the hallmarks of a quantum spin liquid. Application of a magnetic field transverse to the Ising axis introduces both random magnetic fields and quantum fluctuations, which can retard and speed the annealing process, respectively, thereby providing a mechanism for continuous tuning between the destination states. The nonlinear response of the system explicitly demonstrates quantum interference between internal and external relaxation pathways.

Keywords: adiabatic quantum computing; quantum annealing; quantum information; quantum magnetism; random fields.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Chemical Engineering / methods*
  • Magnets / chemistry*
  • Models, Chemical*
  • Quantum Theory*
  • Temperature