Regional dynamics of persistent organic pollutants (POPs) in the Pearl River Delta, China: implications and perspectives

Environ Pollut. 2011 Oct;159(10):2301-9. doi: 10.1016/j.envpol.2011.05.011. Epub 2011 Jun 12.

Abstract

The mass transport budgets of 1,1,1-trichloro-2,2-bis(chlorophenyl)ethane (p,p'-DDT) and decabromodiphenyl ether (BDE-209) in the Pearl River Delta, South China were calculated based on previously collected data. Residual p,p'-DDT, mostly related to historical use, has largely settled into soil (780,000 kg), while the soil BDE-209 inventory (44,000 kg) is considerably smaller. Conversely, large amounts of BDE-209 currently used in numerous commercial products have resulted in a much higher atmospheric depositional flux of BDE-209 (28,100 kg/yr) relative to p,p'-DDT (310 kg/yr). The soil inventory of p,p'-DDT is predicted to decrease to half of its current value after 22 years, and the percent area containing soil p,p'-DDT at levels exceeding the effects range-medium (27 ng/g) will decrease from 40% to 20%. Finally, soil BDE-209 inventory will reach an equilibrium value of 940 tons in ~60 years, when BDE-209 levels in 50% of soil will be above an equivalent risk guideline value (125 ng/g).

Publication types

  • Research Support, Non-U.S. Gov't
  • Review

MeSH terms

  • China
  • DDT / analysis
  • Environmental Monitoring
  • Halogenated Diphenyl Ethers / analysis
  • Insecticides / analysis
  • Organic Chemicals / analysis*
  • Rivers / chemistry*
  • Soil / chemistry
  • Soil Pollutants / analysis
  • Water Pollutants, Chemical / analysis*
  • Water Pollution, Chemical / statistics & numerical data

Substances

  • Halogenated Diphenyl Ethers
  • Insecticides
  • Organic Chemicals
  • Soil
  • Soil Pollutants
  • Water Pollutants, Chemical
  • DDT
  • decabromobiphenyl ether