Ultrafast imaging and the phase problem for inelastic X-ray scattering

Adv Mater. 2010 Mar 12;22(10):1141-7. doi: 10.1002/adma.200904098.

Abstract

A new method for imaging ultrafast dynamics in condensed matter using inelastic X-ray scattering (IXS) is described. Using the concepts of causality and irreversibility a general solution to the inverse scattering problem (or "phase problem") for IXS is illustrated, which enables direct imaging of dynamics of the electron density with resolutions of approximately 1 attosecond (10(-18) s) in time and <1 A in space. This method is not just Fourier transformation of the IXS data, but a means to impose causality on the data and reconstruct the charge propagator. The method can also be applied to inelastic electron or neutron scattering. A general outline of phenomena that can and cannot be studied with this technique and an outlook for the future is provided.

Publication types

  • News
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Algorithms
  • Elasticity
  • Electrons
  • Fourier Analysis
  • Neutrons
  • Scattering, Radiation*
  • X-Rays