The synthesis of polyoxygenated, enantiomerically pure cyclopentane derivatives on route to neplanocin A stereoisomers via alkylidenecarbene species prepared from sugar templates

Carbohydr Res. 2009 Sep 8;344(13):1605-11. doi: 10.1016/j.carres.2009.04.006. Epub 2009 Apr 14.

Abstract

Our new method for the generation of alkylidenecarbenes, based on the reaction of trimethylsilylazide/Bu(2)SnO with alpha-cyanomesylates, has been applied to the synthesis of enantiomerically pure polyhydroxylated cyclopentane derivatives from conveniently functionalized sugar intermediates prepared from D-mannose. The stereoselectivity of the 1,5 C-H insertion reaction leading to the major trans-isomers (8a,b) has been assigned by (1)H RMN spectroscopic data, and correctly rationalized by a computational analysis at DFT level. Compounds 8a and 8b have been designed as suitable intermediates for the synthesis of neplanocin A enantiomer.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adenosine / analogs & derivatives*
  • Adenosine / chemistry
  • Carbohydrates / chemistry*
  • Cyclopentanes / chemical synthesis*
  • Cyclopentanes / chemistry*
  • Magnetic Resonance Spectroscopy
  • Methane / analogs & derivatives*
  • Methane / chemistry
  • Models, Molecular
  • Molecular Conformation
  • Oxygen / chemistry*
  • Quantum Theory
  • Stereoisomerism

Substances

  • Carbohydrates
  • Cyclopentanes
  • carbene
  • neplanocin A
  • Adenosine
  • Methane
  • Oxygen