Picosecond time-resolved laser pump/X-ray probe experiments using a gated single-photon-counting area detector

J Synchrotron Radiat. 2009 May;16(Pt 3):387-90. doi: 10.1107/S0909049509004658. Epub 2009 Mar 20.

Abstract

The recent developments in X-ray detectors have opened new possibilities in the area of time-resolved pump/probe X-ray experiments; this article presents the novel use of a PILATUS detector to achieve X-ray pulse duration limited time-resolution at the Advanced Photon Source (APS), USA. The capability of the gated PILATUS detector to selectively detect the signal from a given X-ray pulse in 24 bunch mode at the APS storage ring is demonstrated. A test experiment performed on polycrystalline organic thin films of alpha-perylene illustrates the possibility of reaching an X-ray pulse duration limited time-resolution of 60 ps using the gated PILATUS detector. This is the first demonstration of X-ray pulse duration limited data recorded using an area detector without the use of a mechanical chopper array at the beamline.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Computer-Aided Design
  • Equipment Design
  • Equipment Failure Analysis
  • Lasers, Solid-State*
  • Photometry / instrumentation*
  • Radiation Dosage
  • Radiometry / instrumentation*
  • Reproducibility of Results
  • Sensitivity and Specificity
  • Transducers*
  • X-Ray Diffraction / instrumentation*