Nanoscale depth-resolved coherent femtosecond motion in laser-excited bismuth

Phys Rev Lett. 2008 Apr 18;100(15):155501. doi: 10.1103/PhysRevLett.100.155501. Epub 2008 Apr 14.

Abstract

We employ grazing-incidence femtosecond x-ray diffraction to characterize the coherent, femtosecond laser-induced lattice motion of a bismuth crystal as a function of depth from the surface with a temporal resolution of 193+/-8 fs. The data show direct consequences on the lattice motion from carrier diffusion and electron-hole interaction, allowing us to estimate an effective diffusion rate of D=2.3+/-0.3 cm(2)/s for the highly excited carriers and an electron-hole interaction time of 260+/-20 fs.