Quantitative electrospray ionization mass spectrometry of zinc finger oxidation: the reaction of XPA zinc finger with H(2)O(2)

Anal Biochem. 2007 Oct 15;369(2):226-31. doi: 10.1016/j.ab.2007.05.019. Epub 2007 May 26.

Abstract

Oxidation plays an important role in the functioning of zinc fingers (ZFs). Electrospray ionization mass spectrometry (ESI-MS) is a very useful technique to study products of ZF oxidation, but its application has been limited largely to qualitative analysis of reaction products. On the other hand, ESI-MS has been applied successfully on several occasions to determine binding constants in metalloproteins. We used a synthetic 37-residue peptide acetyl-DYVICEECGKEFMDSYLMNHFDLPTCDNCRDADDKHK-amide (XPAzf), which corresponds to the Cys4 ZF sequence of human nucleotide excision repair protein XPA, to find out whether ESI-MS might be used quantitatively to study ZF reaction kinetics. For this purpose, we studied oxidation of the Zn(II) complex of XPAzf (ZnXPAzf) by H(2)O(2) using three techniques in parallel: high-performance liquid chromatography (HPLC) of covalent reaction products, 4-(2-pyridylazo)-resorcinol monosodium salt (PAR)-based spectrophotometric zinc release assay, and ESI-MS. Single and double intrapeptide disulfides were detected by ESI-MS to be the sole reaction products. All three techniques yielded independently the same reaction rate, thereby demonstrating that ESI-MS may indeed be used in quantitative kinetic studies of ZF reactions. The comparison of experimental information demonstrated that the formation of the Cys5-Cys8 single disulfide was responsible for zinc release.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Chromatography, High Pressure Liquid / methods
  • Cysteine / chemistry
  • Humans
  • Hydrogen Peroxide / chemistry*
  • Hydrogen Peroxide / metabolism
  • Molecular Sequence Data
  • Oxidation-Reduction
  • Spectrometry, Mass, Electrospray Ionization / methods*
  • Spectrophotometry, Ultraviolet / methods
  • Time Factors
  • Xeroderma Pigmentosum Group A Protein / chemistry*
  • Xeroderma Pigmentosum Group A Protein / metabolism
  • Zinc / chemistry*
  • Zinc / metabolism
  • Zinc Fingers / genetics
  • Zinc Fingers / physiology*

Substances

  • XPA protein, human
  • Xeroderma Pigmentosum Group A Protein
  • Hydrogen Peroxide
  • Zinc
  • Cysteine