N-N splitting of a functionalized mu-eta1:eta2 coordinated N2 ligand leading to a micro-nitrido micro-imido core: mechanistic insight from DFT

Dalton Trans. 2006 Mar 7:(9):1137-40. doi: 10.1039/b514879k. Epub 2005 Dec 23.

Abstract

Silylation of a dinuclear tantalum complex containing a side-on end-on coordinated dinitrogen ligand initiates a sequence of reactions ultimately leading to a bis(micro-imido) structure. DFT is employed to determine the energetics of the entire reaction cascade. Particular emphasis is put on the unprecedented N-N cleavage reaction of the functionalized, micro-eta1:eta2 coordinated dinitrogen ligand. A mechanism for this reaction is derived theoretically and the corresponding transition state is determined.