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Coordination Symmetry Breaking of Single-Atom Catalysts for Robust and Efficient Nitrate Electroreduction to Ammonia.
Cheng XF, He JH, Ji HQ, Zhang HY, Cao Q, Sun WJ, Yan CL, Lu JM. Cheng XF, et al. Adv Mater. 2022 Sep;34(36):e2205767. doi: 10.1002/adma.202205767. Epub 2022 Aug 7. Adv Mater. 2022. PMID: 35841127
Additionally, the cis-coordination splits the Cu 3d orbitals, which generates an orbital-symmetry-matched pi-complex of the key intermediate *ONH and reduces the energy barrier, compared with the sigma-complex generated with other catalysts. ...
Additionally, the cis-coordination splits the Cu 3d orbitals, which generates an orbital-symmetry-matched pi-complex of the key inter …
An Ion-In-Conjugation-Boosted Organic Semiconductor Gas Sensor Operating at High Temperature and Immune to Moisture.
Yu C, He JH, Cheng XF, Lin HZ, Yu H, Lu JM. Yu C, et al. Angew Chem Int Ed Engl. 2021 Jul 5;60(28):15328-15334. doi: 10.1002/anie.202104721. Epub 2021 Jun 9. Angew Chem Int Ed Engl. 2021. PMID: 33885188
Theoretical calculations and in situ FTIR spectra confirmed the ion-in-conjugation-inspired hydrogen bond as key for excellent sensitivity. A NO(2) alarm system was assembled to demonstrate the feasibility of this sensor....
Theoretical calculations and in situ FTIR spectra confirmed the ion-in-conjugation-inspired hydrogen bond as key for excellent sensit …
Built-in Electric Field Triggered Interfacial Accumulation Effect for Efficient Nitrate Removal at Ultra-Low Concentration and Electroreduction to Ammonia.
Sun WJ, Ji HQ, Li LX, Zhang HY, Wang ZK, He JH, Lu JM. Sun WJ, et al. Angew Chem Int Ed Engl. 2021 Oct 11;60(42):22933-22939. doi: 10.1002/anie.202109785. Epub 2021 Sep 14. Angew Chem Int Ed Engl. 2021. PMID: 34431192
This built-in electric field effectively triggers interfacial accumulation of NO(3) (-) ions around the electrocatalyst. The electric field also raises the energy of key reaction intermediate *NO to lower the energy barrier of the rate determining step. ...
This built-in electric field effectively triggers interfacial accumulation of NO(3) (-) ions around the electrocatalyst. The electric field …