Optimization of Thermoplastic Pultrusion Parameters of Jute and Glass Fiber-Reinforced Polypropylene Composite

Polymers (Basel). 2023 Dec 27;16(1):83. doi: 10.3390/polym16010083.

Abstract

Thermoplastic pultrusion is a suitable process for fabricating continuous unidirectional thermoplastics with a uniform cross-section, high mechanical properties due to continuous fiber reinforcement, low cost, and suitability for mass production. In this paper, jute and glass fibers were reinforced with a polypropylene matrix and fabricated using the thermoplastic pultrusion process. The volumetric fraction of the composite was designed by controlling the filling ratio of the reinforcing fiber and matrix. The effects of molding parameters were investigated, such as pulling speed and molding temperature, on the mechanical properties and microstructure of the final rectangular profile composite. The pulling speed and molding temperature varied from 40 to 140 mm/min and 190 to 220 °C, respectively. The results showed that an increase in molding temperature initially led to an increase in mechanical properties, up to a certain point. Beyond that point, they started to decrease. The resin can be easily impregnated into the fiber due to the low viscosity of thermoplastic at high temperatures, resulting in increased mechanical properties. However, the increase in molding temperature also led to a rise in void content due to moisture in jute fiber, resulting in decreased mechanical properties at 210 °C. Meanwhile, un-impregnation decreased with the increase in molding temperature, and the jute fiber began to degrade at high temperatures. In the next step, with varying pulling speed, the mechanical properties decreased as the pulling speed increased, with a corresponding increase in void content and un-impregnation. This effect occurred because the resin had a shorter time to impregnate the fiber at a higher pulling speed. The decrease in mechanical properties was influenced by the increase in void content and un-impregnation, as the jute fiber degraded at higher temperatures.

Keywords: jute/glass fiber reinforced polypropylene; thermoplastic pultrusion; unidirectional hybrid composite.