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Intramolecular Interception of the Remote Position of Vinylcarbene Silver Complex Intermediates by C(sp(3) )-H Bond Insertion.
Díaz-Jiménez À, Monreal-Corona R, Poater A, Álvarez M, Borrego E, Pérez PJ, Caballero A, Roglans A, Pla-Quintana A. Díaz-Jiménez À, et al. Angew Chem Int Ed Engl. 2023 Jan 26;62(5):e202215163. doi: 10.1002/anie.202215163. Epub 2022 Dec 22. Angew Chem Int Ed Engl. 2023. PMID: 36345831 Free PMC article.
The trapping of the elusive vinylogous position of a vinyl carbene with an aliphatic C(sp(3) )-H bond has been achieved for the first time during a silver-catalyzed carbene/alkyne metathesis (CAM) process. ...Density functional theory (DFT) calculations unveil the reaction …
The trapping of the elusive vinylogous position of a vinyl carbene with an aliphatic C(sp(3) )-H bond has been achieved for the first …