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Can a Homometallic Chain Be Ferrimagnetic? This research was supported by CICYT (Grant PB96/0163) and OENB (Grants 6630 and 7967). F.A.M. thanks Prof. C. Kratky and Dr. F. Belaj (Universitat Graz) for the use of experimental equipment. A.E. and R.V. thanks Prof. Dante Gatteschi (University degli Studi di Firenze) for helpful discussions.
Abu-Youssef MA, Escuer A, Goher MA, Mautner FA, Reiß GJ, Vicente R. Abu-Youssef MA, et al. Angew Chem Int Ed Engl. 2000 May;39(9):1624-1626. doi: 10.1002/(sici)1521-3773(20000502)39:9<1624::aid-anie1624>3.0.co;2-7. Angew Chem Int Ed Engl. 2000. PMID: 10820455 No abstract available.
Molybdenum(VI) Bis(imido) Complexes: From Frustrated Lewis Pairs to Weakly Coordinating Cations.
Milinkovic A, Dupé A, Belaj F, Mösch-Zanetti NC. Milinkovic A, et al. Chemistry. 2022 Oct 4;28(55):e202201867. doi: 10.1002/chem.202201867. Epub 2022 Aug 3. Chemistry. 2022. PMID: 35775999 Free PMC article.
Molybdenum(VI) bis(imido) complexes [Mo(NtBu)(2) (L(R) )(2) ] (R=H 1 a; R=CF(3) 1 b) combined with B(C(6) F(5) )(3) (1 a/B(C(6) F(5) )(3) , 1 b/B(C(6) F(5) )(3) ) exhibit a frustrated Lewis pair (FLP) character that can heterolytically split H-H, Si-H and O-H …
Molybdenum(VI) bis(imido) complexes [Mo(NtBu)(2) (L(R) )(2) ] (R=H 1 a; R=CF(3) 1 b) combined with B(C(6) F(5) )(3) (1 a/B(C(6) F …
The value of FDG-PET in the diagnosis of thromboangiitis obliterans--a case series.
Hackl G, Milosavljevic R, Belaj K, Gary T, Rief P, Hafner F, Lipp RW, Brodmann M. Hackl G, et al. Clin Rheumatol. 2015 Apr;34(4):739-44. doi: 10.1007/s10067-014-2648-5. Epub 2014 May 3. Clin Rheumatol. 2015. PMID: 24794493
Different imaging techniques are generally used to exclude potential differential diagnoses. We investigated the value of (18) F-flourodeoxyglucose positron emission tomography ([(18) F]FDG-PET) in the diagnosis of TAO. ...Therefore, increased tracer uptake could be …
Different imaging techniques are generally used to exclude potential differential diagnoses. We investigated the value of (18) F-flou …
Exoseal for puncture site closure after antegrade procedures in peripheral arterial disease patients.
Hackl G, Gary T, Belaj K, Hafner F, Rief P, Deutschmann H, Brodmann M. Hackl G, et al. Diagn Interv Radiol. 2014 Sep-Oct;20(5):426-31. doi: 10.5152/dir.2014.14002. Diagn Interv Radiol. 2014. PMID: 25010369 Free PMC article.
PURPOSE: Exoseal is a vascular clo-sure device consisting of a plug applier and a bio-absorbent polyglycolic acid plug available in sizes 5 F, 6 F, and 7 F. In this study, we aimed to evaluate the effectiveness and safety of the Exoseal vascular closure devic …
PURPOSE: Exoseal is a vascular clo-sure device consisting of a plug applier and a bio-absorbent polyglycolic acid plug available in sizes 5 …
Hydroalkylation of Aryl Alkenes with Organohalides Catalyzed by Molybdenum Oxido Based Lewis Pairs.
Zwettler N, Dupé A, Klokić S, Milinković A, Rodić D, Walg S, Neshchadin D, Belaj F, Mösch-Zanetti NC. Zwettler N, et al. Adv Synth Catal. 2020 Aug 4;362(15):3170-3182. doi: 10.1002/adsc.202000425. Epub 2020 Jun 29. Adv Synth Catal. 2020. PMID: 32982624 Free PMC article.
Three molybdenum(VI) dioxido complexes [MoO(2)(L)(2)] bearing Schiff base ligands were reacted with B(C(6)F(5))(3) to afford the corresponding adducts [MoO{OB(C(6)F(5))(3)}(L)(2)], which were fully characterized. They exhibit Frustrated Lewis-Pairs reactivity when r …
Three molybdenum(VI) dioxido complexes [MoO(2)(L)(2)] bearing Schiff base ligands were reacted with B(C(6)F(5))(3) to afford the corr …
The homologous series of 1,1'-ferrocenylenebisdihalophosphanes (C5H4PX2)2Fe (X = F, Cl, Br, I): precursors for the first metallocene bridged bisphosphaalkene.
Moser C, Orthaber A, Nieger M, Belaj F, Pietschnig R. Moser C, et al. Dalton Trans. 2006 Aug 28;(32):3879-85. doi: 10.1039/b604501d. Epub 2006 Jun 14. Dalton Trans. 2006. PMID: 16896447
A facile synthetic access to the homologous series of 1,1'-ferrocenylene bisdihalophosphanes Fc'(PX2)2 (X = F, Cl, Br, I; Fc' = 1,1'-ferrocenediyl = ferrocenylene = -C5H4FeC5H4-) is reported. ...
A facile synthetic access to the homologous series of 1,1'-ferrocenylene bisdihalophosphanes Fc'(PX2)2 (X = F, Cl, Br, I; Fc' = 1,1'- …
Silanetriols as Powerful Starting Materials for Selective Condensation to Bulky POSS Cages.
Hurkes N, Bruhn C, Belaj F, Pietschnig R. Hurkes N, et al. Organometallics. 2014 Dec 22;33(24):7299-7306. doi: 10.1021/om5010918. Epub 2014 Dec 3. Organometallics. 2014. PMID: 25550679 Free PMC article.
Controlled condensation reactions of tertiary silanetriols CH(3)(CH(2)) (n) (CH(3))(2)CSi(OH)(3) (1b-f; n = 1-5) in the presence of trifluoroacetic acid and the hydrolysis of CH(3)(CH(2))(6)(CH(3))(2)CSiCl(3) (3) lead to the selective formation of the corresponding disilox …
Controlled condensation reactions of tertiary silanetriols CH(3)(CH(2)) (n) (CH(3))(2)CSi(OH)(3) (1b-f; n = 1-5) in the presence of t …
Molecular biodiversity and population structure in common ash (Fraxinus excelsior L.) in Britain: implications for conservation.
Sutherland BG, Belaj A, Nier S, Cottrell JE, P Vaughan S, Hubert J, Russell K. Sutherland BG, et al. Mol Ecol. 2010 Jun;19(11):2196-211. doi: 10.1111/j.1365-294X.2009.04376.x. Epub 2010 Apr 30. Mol Ecol. 2010. PMID: 20465580
There was a clear excess of homozygotes (mean H(O) 0.669, mean H(E) 0.818) and a relatively high F(IS) (mean 0.182), suggests a consistent level of inbreeding or a widespread Wahlund effect in many F. excelsior sites. Gene pool ancestry analysis suggested that the m …
There was a clear excess of homozygotes (mean H(O) 0.669, mean H(E) 0.818) and a relatively high F(IS) (mean 0.182), suggests a consi …
Heterolytic Si-H Bond Cleavage at a Molybdenum-Oxido-Based Lewis Pair.
Zwettler N, Walg SP, Belaj F, Mösch-Zanetti NC. Zwettler N, et al. Chemistry. 2018 May 17;24(28):7149-7160. doi: 10.1002/chem.201800226. Epub 2018 Apr 27. Chemistry. 2018. PMID: 29521459 Free PMC article.
The reaction of a molybdenum(VI) oxido imido complex with the strong Lewis acid B(C(6) F(5) )(3) gave access to the Lewis adduct [Mo{OB(C(6) F(5) )(3) }(NtBu)L(2) ] featuring reversible B-O bonding in solution. ...Single-crystal X-ray diffraction analyses of 2 and 4 …
The reaction of a molybdenum(VI) oxido imido complex with the strong Lewis acid B(C(6) F(5) )(3) gave access to the Lewis adduct [Mo{ …
Halide ligand-more than just sigma-donors? A structural and spectroscopic study of homologous organonickel complexes.
Klein A, Kaiser A, Wielandt W, Belaj F, Wendel E, Bertagnolli H, Zális S. Klein A, et al. Inorg Chem. 2008 Dec 1;47(23):11324-33. doi: 10.1021/ic8007365. Inorg Chem. 2008. PMID: 18959362
The isoleptic organonickel complexes [(bpy)Ni(Mes)X] (bpy ) 2,2'-bipyridine; Mes ) 2,4,6-trimethylphenyl; X ) F,Cl, Br, or I, and for comparison X ) OMe and SCN) have been investigated by multiple spectroscopic means.Their structures have been determined in part by single- …
The isoleptic organonickel complexes [(bpy)Ni(Mes)X] (bpy ) 2,2'-bipyridine; Mes ) 2,4,6-trimethylphenyl; X ) F,Cl, Br, or I, and for …