Dynamics of Correlated Double-Ionization of Two-Electron Quantum Dots in Laser Fields

Materials (Basel). 2023 Feb 7;16(4):1405. doi: 10.3390/ma16041405.

Abstract

Using an ab initio, time-dependent calculational method, we study the non-linear dynamics of a two-electron quantum dot in the presence of ultrashort Thz laser pulses. The analysis of the contribution of the various partial waves to two-electron joint radial and energy distribution patterns revealed strongly correlated electron ejection channels. In the double-ionization process, regardless of the photon energy, the two-electron wave packets are born and remain concentrated until the pulse's peak; at later times, and depending on the photon energy of the field, distinctly different patterns emerge. Our calculations also showed the gradual transition of the radial and energy patterns from a single-peak to a doubly peaked structure, associated with the direct and the sequential double-ionization mechanisms, respectively.

Keywords: ab initio; configuration interaction; double-ionization; energy distributions; quantum dots; radial distributions.

Grants and funding

The Irish Research Council (IRC) for funding this work under the project ID GOIPG/2017/1257. The authors would like to acknowledge partial financing from the COST Action CA18222, “Attosecond Chemisty”.