The anaerobic Escherichia coli ribonucleotide reductase. Subunit structure and iron sulfur center

J Biol Chem. 1996 Apr 19;271(16):9410-6. doi: 10.1074/jbc.271.16.9410.

Abstract

During anaerobic growth Escherichia coli uses a specific ribonucleoside triphosphate reductase for the production of deoxyribonucleoside triphosphates. The active species of this enzyme was previously found to be a large homodimer of 160 kDa (alpha 2) with a stable, oxygen-sensitive radical located at Gly-681 of the 80-kDa polypeptide chain. The radical is formed in an enzymatic reaction involving S-adenosylmethionine, NADPH, a reducing flavodoxin system and an additional 17.5-kDa polypeptide, previously called activase. Here, we demonstrate by EPR spectroscopy that this small protein contains a 4Fe-4S cluster that joins two peptides in a 35-kDa small homodimer (beta 2). A degraded form of this cluster may have been responsible for an EPR signal observed earlier in preparations of the large 160-kDa subunit that suggested the presence of a 3Fe-4S cluster in the reductase. These preparations were contaminated with a small amount of the small protein. The large and the small proteins form a tight complex. From sucrose gradient centrifugation, we determined a 1:1 stoichiometry of the two proteins in the complex. The anaerobic reductase thus has an alpha 2 beta 2 structure. We speculate that the small protein interacts with S-adenosylmethionine and forms a transient radical involved in the generation of the stable glycyl radical in the large protein that participates in the catalytic process.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Anaerobiosis
  • Centrifugation, Density Gradient
  • Chromatography, Gel
  • Electron Spin Resonance Spectroscopy
  • Escherichia coli / enzymology*
  • Glycine
  • Iron / metabolism
  • Iron-Sulfur Proteins / chemistry*
  • Iron-Sulfur Proteins / isolation & purification
  • Iron-Sulfur Proteins / metabolism
  • Kinetics
  • Macromolecular Substances
  • Molecular Weight
  • Ribonucleotide Reductases / chemistry*
  • Ribonucleotide Reductases / isolation & purification
  • Ribonucleotide Reductases / metabolism*
  • Sulfides / metabolism

Substances

  • Iron-Sulfur Proteins
  • Macromolecular Substances
  • Sulfides
  • Iron
  • Ribonucleotide Reductases
  • Glycine