Multiscale Supercrystal Meta-atoms

Nano Lett. 2024 Mar 6;24(9):2758-2764. doi: 10.1021/acs.nanolett.3c04580. Epub 2024 Feb 26.

Abstract

Meta-atoms are the building blocks of metamaterials, which are employed to control both generation and propagation of light as well as provide novel functionalities of localization and directivity of electromagnetic radiation. In many cases, simple dielectric or metallic resonators are employed as meta-atoms to create different types of electromagnetic metamaterials. Here, we fabricate and study supercrystal meta-atoms composed of coupled perovskite quantum dots. We reveal that these multiscale structures exhibit specific emission properties, such as spectrum splitting and polaritonic effects. We believe that such multiscale supercrystal meta-atoms will provide novel functionalities in the design of many novel types of active metamaterials and metasurfaces.

Keywords: Halide perovskites; Mie resonances; exciton-polaritons; supercrystals.