Deep learning assisted XRF spectra classification

Sci Rep. 2024 Feb 14;14(1):3666. doi: 10.1038/s41598-024-53988-z.

Abstract

EDXRF spectrometry is a well-established and often-used analytical technique in examining materials from which cultural heritage objects are made. The analytical results are traditionally subjected to additional multivariate analysis for archaeometry studies to reduce the initial data's dimensionality based on informative features. Nowadays, artificial intelligence (AI) techniques are used more for this purpose. Different soft computing techniques are used to improve speed and accuracy. Choosing the most suitable AI method can increase the sustainability of the analytical process and postprocessing activities. An autoencoder neural network has been designed and used as a dimension reduction tool of initial [Formula: see text] data collected in the raw EDXRF spectra, containing information about the selected points' elemental composition on the canvas paintings' surface. The autoencoder network design enables the best possible reconstruction of the original EDXRF spectrum and the most informative feature extraction, which has been used for dimension reduction. Such configuration allows for efficient classification algorithms and their performances. The autoencoder neural network approach is more sustainable, especially in processing time consumption and experts' manual work.

Keywords: AI classification; Autoencoder neural network; Canvas paintings; Deep learning; Dimension reduction; Pigments; XRF spectra.