Tunable in situ near-UV pulses by transient plasmonic resonance in nanocomposites

Opt Express. 2023 Oct 23;31(22):37275-37283. doi: 10.1364/OE.501153.

Abstract

We propose a concept for generation of ultrashort pulses based on transient field-induced plasmonic resonance in nanoparticle composites. Photoionization and free-carrier plasma generation change the susceptibility of nanoparticles on a few-femtosecond scale under the action of the pump pulse. This opens a narrow time window when the system is in plasmonic resonance, which is accompanied by a short burst of the local field. During this process, frequency-tunable few-fs pulses can be emitted. This paves a way to ultra-compact yet efficient generation of ultrashort pulses at short wavelengths.