Comparison of PM10 emission flux of two fugitive area sources based on the real-time flux monitoring results

Sci Total Environ. 2024 Feb 10:911:168666. doi: 10.1016/j.scitotenv.2023.168666. Epub 2023 Nov 20.

Abstract

Due to a high concentration of particulate matter (PM10), the Korean Peninsula experienced its first poor air quality event of the year between November 19 and November 26, 2021. This study analyzes the reasons behind the occurrence of high-concentration PM10, using the real-time PM10 fugitive emission fluxes and meteorological data measured at two landfills for fly ash of coal-fired power plants located on the west coast. The real-time fugitive emission fluxes of PM10 were estimated at two different locations by a flux-gradient technique based on the eddy covariance method. The measurement results show a weak correlation between PM10 and various meteorological factors in the two places when PM10 levels are low. However, high PM10 concentrations were found to be strongly associated with the relative humidity of site A and the friction velocity of site B, respectively. High emission fluxes were observed at both sites under elevated temperature, high humidity, low wind speed, low frictional velocity, and atmospheric instability. The variation in weather patterns witnessed during periods of high PM10 concentrations in the two locations indicates that the causes of PM10 accumulation are different. The study demonstrates that the gradient-flux method's real-time measurement of fugitive emissions can explain the origin of high PM10 levels and provide essential data to efficiently regulate PM10.

Keywords: 3D sonic anemometer; Atmospheric stability; Light scattering sensor; Monin-Obukhov length; Real-time monitoring.