Research progress on the analysis and application of radioactive hot particle

J Environ Radioact. 2023 Dec:270:107313. doi: 10.1016/j.jenvrad.2023.107313. Epub 2023 Oct 17.

Abstract

Radioactive hot particle is the particulate form of nuclear material that exists in the environment. The U, Pu, Am, Cs, and other radionuclides isotope in the hot particle contain abundant and accurate fingerprint information, such as the origin and age of the nuclear material. The acquisition and analysis of the key information in the hot particle can be equivalent to the analysis of bulk nuclear material, which could directly reflect the real situation of nuclear activities. Therefore, the single particle analysis of hot particles has become an irreplaceable key technology in nuclear safeguards inspection. The rapid identification, screening, locating, and accurate isotope analysis of hot particles from a large number of particles dispersed in environmental media or on the surface of other materials are one of the most important research field in nuclear emergency. In this review, the research process of the analytical methods for hot particles in the last decade was summarized, including the physical character of hot particles, and the techniques of localization, screening, and extraction of hot particles. Furthermore, we also focused on the mass spectrometry technology for the analysis of hot particle. The advantages and disadvantages of the most used mass spectrometry were summarized. Finally, the research trend for hot particle analysis methods was proposed.

Keywords: Extraction; Hot particles; Location; Mass spectrometry analysis; Nuclear safeguards.

Publication types

  • Review

MeSH terms

  • Radiation Monitoring*
  • Radioactivity*
  • Radioisotopes

Substances

  • Radioisotopes