A phenomenological model of the X-ray pulse statistics of a high-repetition-rate X-ray free-electron laser

IUCrJ. 2023 Nov 1;10(Pt 6):708-719. doi: 10.1107/S2052252523008242.

Abstract

Many coherent imaging applications that utilize ultrafast X-ray free-electron laser (XFEL) radiation pulses are highly sensitive to fluctuations in the shot-to-shot statistical properties of the source. Understanding and modelling these fluctuations are key to successful experiment planning and necessary to maximize the potential of XFEL facilities. Current models of XFEL radiation and their shot-to-shot statistics are based on theoretical descriptions of the source and are limited in their ability to capture the shot-to-shot intensity fluctuations observed experimentally. The lack of accurate temporal statistics in simulations that utilize these models is a significant barrier to optimizing and interpreting data from XFEL coherent diffraction experiments. Presented here is a phenomenological model of XFEL radiation that is capable of capturing the shot-to-shot statistics observed experimentally using a simple time-dependent approximation of the pulse wavefront. The model is applied to reproduce non-stationary shot-to-shot intensity fluctuations observed at the European XFEL, whilst accurately representing the single-shot properties predicted by FEL theory. Compared with previous models, this approach provides a simple, robust and computationally inexpensive method of generating statistical representations of XFEL radiation.

Keywords: MHz XFELs; X-ray free-electron lasers; XFELs; computational modelling; correlated fluctuations; dynamic simulations; temporal coherence; time-resolved studies; wavefront propagation.

Grants and funding

Trey Guest acknowledges support from the Commonwealth Scientific and Industrial Research Organization (CSIRO) Alumni. Brian Abbey acknowledges support from the La Trobe Biomedical and Environmental Sensor Technology (BEST) Research Centre. This work has been enabled by megahertz imaging technology developed within internal RD MHz Microscopy and EIC-Pathfinder MHz Tomoscopy (GA 101046448) projects.