At present, self-powered, lightweight, and flexible sensors are widely applied, especially in the fields of wearable devices and human health monitoring. Nevertheless, conventional self-powered flexible sensor systems rely on power supply components such as supercapacitors, nanofriction generators, and solar cells, which present certain limitations, such as high dependence on external environmental factors and the inability to provide long-term stable energy supply. Thus, a paramount exigency emerges for the development of wearable sensors endowed with enduring battery life to enable continuous monitoring of human motion for extended periods. In our academic study, we present an innovative self-powered sensing system that seamlessly combines a pliable zinc-air battery with a strain sensor. This approach offers a stable output signal over extended periods without an external energy device, which is crucial for long-term, continuous human motion monitoring. Through the incorporation of various carbon materials, we realized the multifunction of poly(vinyl alcohol) (PVA)/poly(acrylic acid) (PAA) dual network hydrogels and prepared zinc-air battery electrolytes and strain sensors. Notably, the batteries exhibit impressive power density (82.5 mW cm-2), high open-circuit voltage (1.42 V), and remarkable environmental stability. Even when subjected to puncture and breakage, the batteries remain operational without suffering from electrolyte leakage. Similarly, our strain sensor boasts a broad working range spanning from 0 to 1400%, coupled with a remarkable sensitivity (GF = 2.99) and exceptional capacity to accurately detect various mechanical deformations. When integrated into a single system, the integrated system can monitor human movement for up to 10 h, which has broad prospects in wearable sensor applications.
Keywords: flexible sensor; hydrogel; integrated system; self-powered; zinc−air battery.