Nonlinear field-control of terahertz waves in random media for spatiotemporal focusing

Open Res Eur. 2023 Feb 13:2:32. doi: 10.12688/openreseurope.14508.3. eCollection 2022.

Abstract

Controlling the transmission of broadband optical pulses in scattering media is a critical open challenge in photonics. To date, wavefront shaping techniques at optical frequencies have been successfully applied to control the spatial properties of multiple-scattered light. However, a fundamental restriction in achieving an equivalent degree of control over the temporal properties of a broadband pulse is the limited availability of experimental techniques to detect the coherent properties (i.e., the spectral amplitude and absolute phase) of the transmitted field. Terahertz experimental frameworks, on the contrary, enable measuring the field dynamics of broadband pulses at ultrafast (sub-cycle) time scales directly. In this work, we provide a theoretical/numerical demonstration that, within this context, complex scattering can be used to achieve spatio-temporal control of instantaneous fields and manipulate the temporal properties of single-cycle pulses by solely acting on spatial degrees of freedom of the illuminating field. As direct application scenarios, we demonstrate spatio-temporal focusing, chirp compensation, and control of the carrier-envelope-phase (CEP) of a CP-stable, transform-limited THz pulse.

Keywords: Scattering; genetic algorithm; random medium; spatiotemporal focusing; superfocusing; terahertz; time-domain spectroscopy.

Associated data

  • figshare/10.6084/m9.figshare.19096859

Grants and funding

This project has received funding from the European Research Council (ERC) under the European Union's Horizon 2020 research and innovation programme (grant agreement No 725046). JSTG acknowledges support from The Leverhulme Trust (Leverhulme Early Career Fellowship ECF-2020-537).