PEARS: A Web Tool for Fitting Time-Resolved Photoluminescence Decays of Perovskite Materials

J Chem Inf Model. 2023 Aug 14;63(15):4477-4482. doi: 10.1021/acs.jcim.3c00217. Epub 2023 Jul 18.

Abstract

Time-resolved photoluminescence (TRPL) is a powerful tool to investigate charge carrier recombination processes in emissive materials. Perovskite materials are extremely promising for applications in solar cells; however, the interpretation of their TRPL is arduous due to the complicated nature of the recombination processes occurring in these materials. We present here the PErovskite cArrier Recombination Simulator (PEARS) web tool for effortlessly and quickly fitting TRPL of perovskite materials using advanced charge carrier recombination models, allowing for the extraction of recombination rate constants and trap state concentration. PEARS is flexible and can adapt to different situations, by ignoring recombination processes or fixing known parameters (e.g., the doping concentration). The tool is publicly available at https://pears-tool.herokuapp.com.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Calcium Compounds
  • Oxides
  • Pyrus*

Substances

  • perovskite
  • Calcium Compounds
  • Oxides