Combining Satellite-Derived PM2.5 Data and a Reduced-Form Air Quality Model to Support Air Quality Analysis in US Cities

Geohealth. 2023 May 9;7(5):e2023GH000788. doi: 10.1029/2023GH000788. eCollection 2023 May.

Abstract

Air quality models can support pollution mitigation design by simulating policy scenarios and conducting source contribution analyses. The Intervention Model for Air Pollution (InMAP) is a powerful tool for equitable policy design as its variable resolution grid enables intra-urban analysis, the scale of which most environmental justice inquiries are levied. However, InMAP underestimates particulate sulfate and overestimates particulate ammonium formation, errors that limit the model's relevance to city-scale decision-making. To reduce InMAP's biases and increase its relevancy for urban-scale analysis, we calculate and apply scaling factors (SFs) based on observational data and advanced models. We consider both satellite-derived speciated PM2.5 from Washington University and ground-level monitor measurements from the U.S. Environmental Protection Agency, applied with different scaling methodologies. Relative to ground-monitor data, the unscaled InMAP model fails to meet a normalized mean bias performance goal of <±10% for most of the PM2.5 components it simulates (pSO4: -48%, pNO3: 8%, pNH4: 69%), but with city-specific SFs it achieves the goal benchmarks for every particulate species. Similarly, the normalized mean error performance goal of <35% is not met with the unscaled InMAP model (pSO4: 53%, pNO3: 52%, pNH4: 80%) but is met with the city-scaling approach (15%-27%). The city-specific scaling method also improves the R 2 value from 0.11 to 0.59 (ranging across particulate species) to the range of 0.36-0.76. Scaling increases the percent pollution contribution of electric generating units (EGUs) (nationwide 4%) and non-EGU point sources (nationwide 6%) and decreases the agriculture sector's contribution (nationwide -6%).

Keywords: NAAQS; decision‐making; environmental justice; fine particulate matter; reduced‐form model; satellite‐derived PM2.5.